Method of controlling the internal structure of matter

ABSTRACT

A method for molding is disclosed in which a fluent molding material is flowed into a cavity of a mold, which is then shaped into a configuration defined by the mold. Control signals which are applied by operating a master controller to control the transfer of heat with respect to the molding material, in order to predeterminately control the temperature of the molding material as it flows into and is retained within the mold. The temperature of the molding material flowed into the cavity is sensed, and feedback signals are generated relating to the sensed temperature. The feedback signals are compared to reference signals indicative of a desired molding material temperature and a further control signal is generated which is applied to control the variables of the molding operation, including the temperature of the molding material.

RELATED APPLICATIONS

This is a continuation of Ser. No. 027,075, filed Mar. 17, 1987,abandoned, which is a continuation of Ser. No. 535,545, filed Sep. 26,1983, abandoned, which is a continuation of Ser. No. 278,399, filed Jun.29, 1981, abandoned, which is a continuation of Ser. No. 663,243, filedMar. 3, 1976, now U.S. Pat. No. 4,288,398, which is a continuation ofSer. No. 372,838, filed Jun. 22, 1973, abandoned; above-mentioned Ser.No. 278,399 is also a continuation-in-part of application Ser. No.950,017, filed Oct. 10, 1978, now U.S. Pat. No. 4,318,874, which is acontinuation of Ser. No. 483,037, filed Jun. 25, 1974, now U.S. Pat. No.4,120,922, which is a continuation of Ser. No. 297,452, filed Oct. 13,1972, now U.S. Pat. No. 3,820,928, which is a continuation of Ser. No.849,014, filed Aug. 11, 1969, now abandoned which is acontinuation-in-part of Ser. No. 721,401, filed Apr. 15, 1968, now U.S.Pat. No. 3,616,495, which is a continuation-in-part of fourapplications: (1) Ser. No. 142,405, filed Oct. 2, 1961, now U.S. Pat.No. 3,422,648, which is a continuation-in-part of Ser. No. 691,622,filed Oct. 22, 1957, now U.S. Pat. No. 3,002,615, (2) Ser. No. 421,817,filed Dec. 29, 1964, now U.S. Pat. No. 3,462,524, (3) Ser. No. 421,860,filed Dec. 29, 1964, abandoned, and (4) Ser. No. 439,549, filed Mar. 15,1965, abandoned, which is a continuation-in-part of Ser. No. 734,340,filed May 9, 1958, now U.S. Pat. No. 3,170,175; above-mentioned Ser. No.483,037 is also a continuation-in-part of Ser. No. 416,219, filed Nov.15, 1973, now abandoned which is a continuation of Ser. No. 194,630,filed Nov. 1, 1971, abandoned, which is a continuation-in-part of Ser.No. 721,401, above.

This invention relates to an apparatus and method for forming moldablematerials including such materials as thermoplastic and thermosettingpolymers, metals, certain ceramic materials and composite materialswhich may be formed to shape in a mold or die such as an injection mold,die casting mold, continuous casting mold or extrusion die wherein thematerial is introduced therein or processed to shape in a molten orflowable condition such that it may be caused to crystalize or otherwiseform a defined internal structure as, or shortly after, it attains itsmolded shape.

During the formation of many materials such as metals or polymers from amolten or plastic condition, imperfections frequently form in thematerial such as surface irregularities, cracks, internal occlusions orflaws, porosity due to the formation of gas pockets, etc. The strengthof materials formed by conventional techniques is often substantiallyless than that which may be obtained due not only to the formation ofsurface and internal flaws but also to the fact that the internalstructure of the material, such as its crystalline structure, isfrequently imperfect. Such imperfections may result from the lack ofcontrol of the growth and formation of crystals, such as metal crystals,due to disorientation thereof or the size and arrangement of spherulitescommon in many polymers.

Accordingly, it is a primary object of this invention to provide anapparatus and method for improving the structures of various articles ofmanufacture formed from a molten or plastic state by predeterminatelycontrolling the formation of such articles including their internalcharacteristics, such as crystal growth and orientation, spheruliteformation and the like by the application of controlled wave energy tothe solidifying or forming material, such as ultrasonic energy,induction energy, shockwaves and magnetic fields applied per se or incombination with one of the other forms of such energy to thesolidifying material.

Another object is to provide an improved apparatus and method forcontrolling the solidification of a material in a mold by applyingsharp, intermittent forces to the material as it solidifies.

Another object is to provide an apparatus and method for controlling theinternal structure of an article by means of an intense magnetic forceapplied to the article solidification.

Another object is to provide an improved method of enhancing thestrength of metals by use of an intense magnetic field to controlcrystal growth.

Another object is to provide a method of improving and enhancing thestrength of a material such as a polymer by the application of one ormore of the forces of magnetism, sound such as ultrasonic energy andintense vibrations applied directly to the material as it solidifies.

Another object is to provide a method for improving the internalstructure of molded plastic or metal articles by the combined forces ofmagnetism and ultrasonics applied thereto in a predetermined manner asthe material solidifies.

Another object is to provide an improved method for controlling theinternal structure and crystal growth within the continuously shapedarticle such as an extrusion or continuous casting formed from a moltenor semi-molten metal such as a melt or supply of powdered metal renderedmolten or semi-molten.

Another object is to provide an apparatus and method for controlling theshape and internal structure of an article as it is molded by applying ashockwave or plurality of shockwaves to the material during one or morepredetermined times in the molding cycle.

With the above and such other objects in view as may hereafter morefully appear, the invention consists of the novel constructions,combinations and arrangements or parts as will be more fully describedand illustrated in the accompanying drawings, but it is to be understoodthat changes, variations and modifications may be resorted to which fallwithin the scope of the invention as claimed.

In the drawings:

FIG. 1 is a cross-sectional view of male and female components of a moldand illustrating transducing means associated with the walls of the moldcomponents;

FIG. 2 is a cross-sectional view of a modified form of the mold assemblyof FIG.1;

FIG. 3 is a cross-sectional view of a fragment of a mold havingelectrical transducing means surrounding at least a portion thereof;

FIG. 4 is a cross-sectional view of a fragment of a mold havingtransducing means about the mold and secured within the wall of themold;

FIG. 5 is a cross-sectional view of a fragment of a continuous castingmold having transducing means surrounding a portion thereof;

FIG. 6 is a schematic diagram illustrating an automatic control systemoperative to control both molding and transducing means of the typesshown in FIGS. 1-5;

FIG. 7 shows portions of a control system for casting apparatus of thetype shown in FIG. 5; and

FIG. 8 is a schematic diagram of a modified form of the control systemof FIG. 6 and applicable for controlling a molding, casting or extrusionprocess employing the molds of FIGS. 1-6 for modifications thereto asillustrated in FIG. 8.

In FIG. 1 is shown part of a molding apparatus 10 including a first moldmember 11 operative to close with a second mold member 20 to define avolume V therewith in which volume molding material may be formed toshape from a molten or flowable condition. The mold member 11 has a baseportion 12 with a surface 13 for engaging a rim or flange portion 22 ofthe second mold member 20 when either or both said members are urgedtogether for sealing the volume V upon closure of the mold. Mold member12 is shown having a nose portion 14 projecting into volume V fordefining, for example, the interior surface of a molding, forging orextrusion formed in the mold. A number of separate components areutilized in the assembly of mold member 12 to define a plurality ofpassageways in the nose portion 14 and/or the base portion 12 thereof. Afirst passageway 15 is shown extending in a helical path through noseportion 14 and in any suitable path in the base portion 12 of the moldfor flowing a heat transfer fluid therethrough during any suitable timein a molding cycle by controlling the operation of a valve or pump foreffecting said flow. While the fluid is preferably one which isoperative to receive heat from the mold wall transferred thereto fromthe molding material and to rapidly remove said heat so as to permit themolding to rapidly solidify, said passageway 15 may also be operative tocarry a heated fluid if it is desired to melt or cure molding materialpreviously disposed in the molding cavity V.

A second passageway, or passageways extend in a suitable formationthrough the nose portion 14 of the mold and contain one or moreelectrical conductors 17 which may comprise resistance heating elements,an induction coil or electrical magnet coils operative to perform on themolding material as hereafter described. The passageway or passageways16 which contain the electrical conductors 17 preferably also extendthrough the base portion 12 of the mold near surface 13 thereof toopenings in the mold member 11 and then to a source of intenseelectrical energy for energizing the electrical member or members insaid passageways 16.

Mold member 20 has a side wall 21, a bottom wall 23, and a flange 22circumscribing the side wall. The side and bottom walls, as well as theflange of the mold member 20, are shown having a plurality ofpassageways 25 and 26 extending in any suitable path therethrough.Passageway 25 is operative to receive and flow a heat transfer fluidthrough the wall of the mold for effecting heat transfer operationsrelative to the material being molded and passageway 26 contains one ormore electrical conductors therein which connect to a source ofelectrical energy for energizing same so as to heat by resistance orinductance the material in the cavity V or to apply an intense magneticforce thereto for affecting the molding material as it solidifies in themanner described. The conductors 27 and 17 of FIG. 1 may compriseelectrical resistance heating elements, or one or more coils ofconventional wires or superconducting material operative when energized,to generate a magnetic field of the desired intensity in and surroundingthe material being molded, forged or sintered to shape in the cavity ofthe mold.

In further embodiments of apparatus of the type shown in FIG. 1, thenose member 14 may comprise a removable probe operative to merelysubject the molding material in the mold to vibrational, induction ormagnetic energy during a portion of the molding cycle so as to affectthe material's crystal growth as described but removable from themolding prior to complete formation or solidification thereof whichformation may be effected solely in the mold 20 per se, by advancinganother mold member thereagainst while in mold member 20 or by removalof the semi-solidified casting and the further molding or forgingthereof.

Both mold members 14 and 20 are illustrated as being made up of aplurality of sections which, upon assembly, define the electrical andfluid passageways therein. The mold member or nose 14, for example, ismade of at least two sections 18 and 18' each being tubular with thesection 18 being hollow and defining a passageway 19 extendingcompletely through the nose member or portion 14 and communicating withthe molding cavity volume V'. Passageway 19 may be utilized for flowingor injecting molding material into the mold cavity volume and/or toserve one or more other functions. For example, passageway 29 may serveas means for applying shock waves or ultrasonic vibrations to themolding material in one or more manners. A fluid, other than moldingmaterial such as air or gas injected into passageway 19 may be pulsed orhave shock waves generated therein which are transmitted aftertravelling down said passageway to the molding material immediatelyadjacent the end of nose 14 while 14 is fully inserted and/or during theremoval of nose 14 from the solidifying molding material. A transducer,such as one made of a pietzo-electric material such as barium titanate,lead sirconate or other suitable material which will vibrate in theultrasonic range when energized by high frequency electrical signals,may be disposed in passageway 19 at or near the end thereof andprotected from the corrosive effects of the molding material by one ormore means such as a metal plug at the end of passageway 19 and/or heattransfer fluid conducted through the passageways in the nose member 14thereto.

The device of FIG. 1 may be utilized to mold and/or improve the internalstructure of a variety of materials including metals, polymers andceramics as well as composite materials by the application of one ormore of the described forces of high amplitude, low frequency magneticor sound vibrations, high frequency sound vibrations in the ultrasonicrange (above 20 kilocycles), magnetic forces such as generated by one ormore induction coils employing super-conducting magnetic wire or othersuitable means disposed in the walls of mold members 14 or 20 and/orcontrolled heating resulting from one or more induction coils disposedin said walls of said mold components.

Further variations in the apparatus of FIG. 1 as well as the otherembodiments to be described include the use of a plurality of spacedapart probes of the type defined by notation 14 which protrude into amold, casting or extrusion die and are operative to simultaneously orsequentially generate one or more forms of energy and transmit same tothe solidifying molding material for controlling crystal growth,orientation, grain refinement or any of the described variables. Suchprobe or probes may be fixed with respect to one die member or movableto retract from the molding, casting or forging as it solidifies so thatsaid molding, casting or forging may be further worked by the dies orshaped in a manner other than that defined by the shape of the probe orprobes. In other words, the probe or probes may be used for the combinedfunction of shaping the material disposed thereagainst and affecting itsinternal structure or merely as a means for affecting its internalstructure. The induction, magnetic or magnetodtrictive coil meansdisposed in the probe may be operated at a fixed intensity or power andfrequency, or at a power level and frequency which predeterminedlyvaries during a molding cycle. Also, plural coil means and/or transducermeans disposed in the mandrel or mold nose 14 and/or the wall of theouter mold member 20 may be separately energizable and energized in anydesired sequence or at different predetermined power levels orfrequencies during a molding cycle.

In FIG. 2 is shown a modified form of the invention including moldingapparatus 30 comprising a male mold member 31 and a female mold member40 defining a molding cavity V' therebetween in which material may beinjection molded, cast, forged, extruded, pressed or otherwise formed toshape from a molten, plastic or fluent condition. The male mold member31 includes a base 32 having a surface 33 operative to sealingly engagethe outer surface 41 of the female mold member 40. Notation 34 defines anose portion of the male mold member which projects into the moldingcavity of the female mold member and may be any suitable shape operativeto define the inside surface of the molded article while the outersurface of said article is defined by the cavity surface 44 of member40. Member 40 has a side wall 42 and a bottom wall 43 and may be of anysuitable shape and structure. Nose portion 34 of male mold member 31contains one or more coils 36 of a conducting metal or superconductorwhich coil may be utilized for induction heating the molding material orgenerating an intense magnetic field therein as said material solidifiesfor the purpose of affecting the internal structure of said material asdescribed. The passageways or cavity 35 in the nose portion 34 areillustrated as cylindrical in shape and preferably has one or morepassageways extending therefrom through the base portion 32 of the moldmember 31 for connecting the wires 36 of the coil formation 37 with asource of energizing electrical potential. Also illustrated are one ormore passageways 37 which extend through the nose portion 34 of moldmember 32 for conducting a heat transfer fluid relative to the moldingmaterial and/or for admitting molding material to the cavity moldingvolume V'.

Mold member 40 is also illustrated as being hollow and containing one ormore passageways 45 in the side wall 42 and/or bottom wall 43 thereof.Disposed in the passageways 45 are a plurality of conductors shaped asmagnetic induction or heating coils 47 operative to affect the physicalproperties of the molding material as it solidifies by, for example,controlling crystal growth or the like.

It is noted that the mold structure of FIG. 2 may be subject to furthermodification wherein the nose member 34 of the male mold member 32contains or is coupled to one or more ultrasonic transducers or meansfor vibrating the mold member and the nose 34 thereof at any suitablefrequency including vibrations in the ultrasonic range operative tophysically affect and improve the material being molded just as andimmediately after it solidifies.

If the coil devices 47 disposed within the cavity 45 of the female mold42 and/or those 36 disposed in the mandrel 34 of the male mold member 32define super conducting magnets, then they may be utilized to causeexpansion and partial reduction in the dimensions of the respective moldmembers or portions thereof sufficient to impart blows or compressiveforces to material which is disposed within the mold cavity volume V'which may be substantially useful in affecting crystal structure andorientation assuming that said material initially completely fills theclosed-off mold cavity.

By injecting molding material into the mold cavity volume V' atsubstantial pressure and retaining said pressure while either or boththe walls of member 42 and mold member 34 are intermittently expandedand partially collapsed to increase and decrease the volume V', thematerial solidified, being extruded or compression molded in said moldcavity may be substantially affected as to its structure by, forexample, increasing the density thereof, eliminating or substantiallyreducing porousity, controlling, crystal growth and orientation.

Whereas the apparatus of FIGS. 1 and 2 provides means located within oneor more mold components for coupling electromagnetic or induction energyto material disposed in the cavity of a mold, FIG. 3 illustrates part ofa molding apparatus 50 having energy coupling means 55 situated outsideof the mold but coupled to the wall thereof. The apparatus 50 includes amold or die component 51 which may be one of a plurality of assembleablecomponents operative to define a mold cavity 54 in which formablematerial is cast, pressed or otherwise shaped to conform to the wallthereof. The mold member 51 is shown as having a circumscribing sidewall 52 and a bottom wall 53. Coupled to the bottom wall 53 is shown atransducer 55 such as an electrically excitable piezo electrictransducer or other type of electrically excitable device operative,when electrically energized by applying the proper electrical energy toan input line 56 extending thereto, to generate and transmit vibrationalenergy such as ultrasonic waves to the wall 53 and therethrough tomaterial disposed in the molding cavity 54 before said material hascompletely set or solidified so as to affect the internal structure ofsaid material by orienting the crystals thereof and, in certaininstances, by otherwise affecting crystal growth in a manner such as toprovide a uniform or predetermined crystalline structure by the time thematerial has solidified. The transducer 55 may also be operative toimprove the characteristics of the surface strata of the material formedin the molding cavity as well as to facilitate removal of said materialfrom said cavity and is shown mounted on the drop-out door 56 of themold.

Also illustrated in FIG. 3 is an assembly 57 which includes a pluralityof coil windings 58 of insulated wire such as copper or any suitablesuperconductor which extend around the mold member 51 and are operativewhen energized to affect the material molded in cavity 54 in either orboth of two manners. In a first manner of operation of the coil member57, electrical energy transmitted thereto through an input line 54 isoperative to induction heat and melt or otherwise affect materialadmitted to the molding cavity 54. In a second mode of operation, theenergized transducer or coil located within member 57 is operative togenerate an intensive magnetic field and is intermittently energized soas to create and collapse said field at a predetermined frequency forpredeterminedly affecting the material being molded, cast or extruded inthe mold or die member 51. If the member 57 is a superconductingelectro-magnet, it may be operative in one or more modes such as, (a)control crystal growth, (b) orient crystals formed within the materialdisposed within cavity 54, (c) compact material disposed within 54 byaffecting the dimensions of the mold cavity by causing the walls 51 ofthe mold to come closer together, (d) apply intermittent forces to themolding material by vibrating or reducing and expanding the crosssectional area of the mold cavity by means of magnetic forces applied tothe wall of the mold, (e) applying impact forces by magnetic means tothe wall of the mold and the material therein to affect crystalformation and orientation as well as to eliminate or reduce porousity inthe molded material. By adding material to the mold when the magneticfield is removed and restraining said material so as to prevent the flowof same while a magnetic field is so applied, the density of a membermolded within cavity 54 may be increased when compared with the densityof such material molded without use of the electro-magnetic forcegenerating means 57. The effect of such intense magnetic field on themold itself may serve to reduce the volume of the mold cavity so as tocompress the molding material while it is solidifying to increase itsdensity, control or eliminate porosity, control crystal formation andgrowth, orient said crystals, etc. PG,18

In another form of the invention, molding apparatus of the typedescribed may be utilized for molding particulate or powder materialswith or without the application of induction, sonic or magnetic energyfor predeterminately affecting the crystalline or grain structure of thearticles so formed. For example, induction and/or resistance heatingcoils means may be provided within or about either or both of theassembled mold members and operative to heat the mold walls andparticulate material disposed in the molding cavity. If the particulatematerial is a thermoplastic polymer or thermosetting resin which iscured by heat, the walls of either or both mold members may beinductively or resistance heated to effect melting of the charge and/orthe curing thereof by heat transfer thereto through the walls of themold. If the particulate material is metal powder such as aluminumpowder, a predetermined quantity thereof may be charged into a moldcavity prior to or after assembly of the mold members and may be heatedto a molten or semi-molten condition by energizing one or more inductioncoils disposed in one of the manners hereinabove described andillustrated in the accompanying drawings. Compositions of metal and/orceramic powders with filaments such as metal whiskers may be chargedinto a mold, compressed and/or inductively heated to form a compositearticle and allowed to solidify by removal of the induction energy withor without the further application of force as described to affect theinternal structure of said composite article.

In another form of the invention, one or more of the components of themold may be heated by resistance heating elements disposed in or aboutthe mold wall while other coil formations may be operative to generateinduction energy in the particulate and/or whisker elements disposed inthe mold as molding material to cause same to become molten orsemi-molten while, an auxiliary magnetostictive electrical device orultrasonic transducer may be operative at the proper interval during amolding cycle to impart ultrasonic vibrations to the material beingmolded through the wall or walls of either or both mold members forgreater enhancing the physical strength thereof such as by crystalorientation and improvement of grain boundary structure. As hereinbeforedescribed, magnetic or vibrational energy may be so applied to thematerial being molded while it is in a semi-molten condition or justprior to the formation of the crystalline structure thereof so as toorient and predeterminately affect said structure and crystal growth.

A combination of relatively low amplitude ultrasonic vibrations andlarger amplitude sub-ultrasonic vibrations may be simultaneously orsequentially applied to either or both mold members for transmission tothe material being molded to as to beneficially affect the crystalstructure of the material being molded during the latter stages of theformation thereof and either or both these techniques may be combinedwith the application of an oscillating magnetic field to the moldmembers and molding material disposed therebetween.

FIG. 4 shows a modified form of the invention wherein an ultrasonictransducer of the type described or any of the hereinbefore describedelectrical energy transducing means, is shown embedded or otherwisesecured within the wall 53' of a mold 50' which is made as described. Insuch a construction, not only is the transducer protected by the wall ofthe mold from external blows, but it is positioned, as a result of beingencapsulated or secured within the mold wall, much closer to the surfaceof the molding cavity, thereby resulting in substantially lessattenuation than would be experienced if the transducer were operativeto transmit wave energy completely through the entire thickness of themold wall. In the operation of the apparatus of FIG. 4, as in theoperation of the hereinbefore described apparatus, the combined effectsof ultrasonics and intense magnetic fields may be utilizedsimultaneously or in sequence to improve the characteristics of thecasting or molding.

In FIG. 5 is shown apparatus of the type described applied to acontinuous casting mold 60 the upper end of which is illustrated justbelow the ladle (not shown) which is operative to feed molten metal tosaid mold. The mold is shown as having a side wall 61 with one or morepassageways 62 therein for flowing heat transfer fluid through the moldduring the continuous formation and downward travel of a casting C shownexiting from the open end 64 of the mold cavity or passageway 63extending completely through the mold or die 60. Intense ultrasonicwaves are generated by one or more transducers provided in one or morehousings 65 completely or partially surrounding the side wall 61 of themold 60. Said housing 65 may also contain one or more super-conductingmagnetic coils and lead-in wires extending from a source of suitableelectrical energy for energizing said coils and generating a timevarying intense magnetic field in the mold wall and through the moldingmaterial in the volume thereof containing semi-molten and solidifyingmaterial so as to predeterminedly affect grain structure, crystal growthand crystal orientation within the continuously cast rod or billet. Theportion of the continuous casting mold 60 illustrated in FIG. 5 includesmetal in a solid phase near the bottom end of the mold and in asemi-molten and molten phase near the upper end of the mold.Accordingly, the ultrasonic energy and/or intense variable oroscillating magnetic field is generated in the region which includes thesolidifying phase of the casting so as to beneficially affect theinternal structure of the casting as hereinbefore described.

Apparatus is illustrated in FIG. 6 for controlling variables of thehereinbefore described molding apparatus. The control system 70 includesa multi-circuit controller 71 comprising a computer, tape or cardreader, multi-circuit timer or the like operative to generate a sequenceof signals at predetermined time intervals during a controlled cycle, orsignals resulting from internal computations of the device 71 on aplurality of outputs 72 thereof which extend to various switches, valvesand controls as hereinafter described.

A control cycle is initiated when molding material is admitted to themold or die 69 which may comprise any of the hereinbefore describedmolds or dies. The material may be poured into the mold 69 from the openend thereof or injected through the opening in nose member or nozzle 68disposed in or just above said die. Assuming that member 68 is both aninjection nozzle and a probe operative to transmit ultrasonic or otherforms of energy to the molten material in the mold, a charge of themolding material is admitted to the passageway 68' in 68 through aninlet line 81 connected to a supply of said material (not shown) througha valve 82 which is solenoid or servo motor operated. The solenoid orservo motor for valve 82 is activated by a signal generated by thecontroller 71 to close and admit molding material to the mold 69. Priorto or just after admission of the complete charge to the mold or die 69,the mandrel or probe 68 may be lowered into the melt for the purposesdescribed by means of a servo motor 76 which is controlled in bothforward and reverse directions by signals generated by controller 71 andwhich has its output shaft 78 coupled to a spur or worm gear 79 which iscoupled to a suitable gear 80 extending upwardly from member 68 to urgethe downward and upward thereof depending on the operation of servo 76.

With the projection of mandrel or probe 68 into the melt, the describedtransducing means mounted therein may be energized by activation of anormally open switch 73, by a signal from controller 71 connecting asource 74 of suitable electrical energy to the input line 75 extendingto the transducing means in probe 68. The transducing means located insaid probe then operates in the manner described to effect suitablecontrol of the solidifying molding material and transducing meanslocated in the mold member 69, as described, may also be energized byclosing a second normally open switch 85 disposed between the input lineto the transducing means in the mold wall and a suitable source ofelectrical energy. Also illustrated in FIG. 6 are valve means 84 and 87for controlling the flow of heat transfer fluid through lines 83 and 86extending respectively to the passageways in the probe 68 in the moldwall 69. Predeterminedly controlling the flow of heat transfer fluid inboth the probe and the mold wall may be effected to predeterminedlycontrol crystal growth and solidification of the casting or molding in apredetermined manner concurrent with the predetermined control of theoperation of the transducing means. In other words, since thetransducing means is operative at a predetermined time during thesolidification of the molding in the mold, and since the rate of flow ofheat transfer fluid is directly proportional to the manner in whichsolidification occurs, control of both these variables should be theresult of programming the means for varying same preferably in a closedloop control cycle which includes means for measuring temperature orother variables associated with the molding or casting and generatingfeedback signals to be bucked a standard signal or a signal which variespredeterminedly with time during the cycle.

While the apparatus of FIG. 6 is illustrated as being substantially anopen loop control system, FIG. 7 illustrates means for closing the loopby scanning a portion of a casting such as the continuous casting C ofFIG. 5 with an X-ray means. The apparatus includes an X-ray generatingtransducer located in the housing 90 for generating and passing X-raysalong a path 91 completely through the casting C which are picked up bya receiver 92 located across the other side of the casting and operativeto generate an output signal which varies in accordance with variationsin the internal structure of the casting. The output signal is passed toa comparator device 93 such as a summing amplifier which receives areference signal on a second input 94 thereto and the output 95 or 93 isan error signal which may be passed to the computer located within thecontroller 71 which may be an adaptive device operative to adjust orvary the duration of signals generated on the output of the device andpassed to the various controls for controlling the variables described.

In temperature sensing apparatus, the X-ray generating means located inhousing 90 may be eliminated if the device situated in housing 92 is aninfra-red scanner operative to soan the continuous casting C andgenerate on its output a signal which varies in proportion to variationsin temperature of said casting so as to provide a signal to comparatordevice 93 which is bucked against a reference signal generated on input94 for providing a error signal on the output 95 thereof. The resultingerror signal may be used to correct one or more of the output signalsgenerated by the computer in device 71 of FIG. 6 for correcting, forexample, the rate or duration of flow of heat transfer fluid, durationor intensity of energy utilized to energize one or more of thetransducers described, rate of flow of molding or casting material,location of the probe or mandrel 68, etc.

FIG. 8 illustrates a control system applicable to the apparatushereinbefore described whereby a plurality of forms of transducing meansare provided in coupling relationship with the mold components and maybe operative per se, in sequence or concurrently during one or moretimes in a molding, casting or extrusion process to predeterminatelyaffect and control the molded or extruded article.

The apparatus of FIG. 8 includes a mold assembly 98 which is illustratedas composed of a mold 99 having a side wall 100 containing a pluralityof passageways therein denoted 101, through which passageways flow aheat transfer fluid for controlling the rate of solidification of themolding material in the mold. While the mold of FIG. 8 is illustrated asclosed at its lower end, it may be designed in accordance with any ofthe structures hereinbefore described and may include, in addition to acasting mold as illustrated, an injection mold for molding syntheticpolymers or metal under pressure, a die-casting mold, a continuouscasting mold open at the lower end for continuously downwardly castingelongated shapes or an extrusion die through which metal, plastic orceramic materials may be continuously forced and formed to shape or acompression mold for shaping molten or particulate material.

The mold 99 is illustrated as open at the upper end, although it maycontain a closure means of the type described, and is shown having aprobe 104 movable from a position above the mold into the moldingmaterial or melt disposed in the mold cavity 103. A pouring spout 117 isdisposed over the mold cavity for flowing or injecting a predeterminedquantity of molding material therein. Molding material is flow-regulatedby means of a valve 118 and pump 118' disposed between a reservoir ofmolding material and the spout 117. The pump 118 is controlled by a gearmotor 120 having on and off controls 120F and 120S which are connectedto a master controller 134 to be described.

The probe 104 is shown movably supported in a lineal bearing 104B whichis supported above the mold on a mount 104M which is supported by thesame frame or mount supporting the mold. A passageway 106 extendinglongitudinally through the probe 104 contains wires for conductingelectrical energy of suitable frequency and amplitude to a plurality oftransducers disposed within the probe. One transducer 125 is shownsecured within the lower end portion of the probe 104 and may comprisean ultrasonic transducing means such as one or more formations of bariumtitanate or lead zirconate as described and properly mounted within theprobe to predeterminately radiate ultrasonic vibrations through theprobe wall and outwardly therefrom. A second transducer 128 is alsomounted within a cavity 128C in the probe wall and mounts one or morecoils of wire which operate, as described, to impart magnetic orinduction fields to the molding material surrounding the probe.

A passageway 105 extends through the probe wall for conducting heattransfer fluid therethrough to protect the probe and the transducingmeans mounted therein from heat damage.

Notation 107 refers to a fluid coupling connecting the passageway orpassageways 105 with a flexible metal hose lines defining twopassageways for conducting heat transfer fluid to and from thepassageways in the probe. A pump 114 driven by a gear motor is operativeto predeterminately flow heat transfer fluid to and from the probepassageway 105 through flexible lines 112 and 113. The pump 114 isoperated by a gear motor 115 having on and off controls 115F and 115Swhich are respectively controlled by the master controller 134.

A second pump 121 is operatively connected through an output line 123 toa passageway 101 extending through the wall 100 of the mold forcontrolling heat transfer fluid flow and solidification of moldingmaterial disposed in the mold cavity 103. The pump 121 is operated by agear motor 122 having on and off controls respectively designated 122Fand 122S which are also controlled by signals generated by the mastercontroller 134. Notation 124 refers to a reservoir for supplying heattransfer fluid to the pumps 121 and 114.

The probe 104 is predeterminately positioned within the mold cavity 103and either retained therein during an entire molding procedure, variedin its location during the molding procedure or removed therefrom priorto complete solidification of the molding material by a positioningarrangement which includes a reversible gear motor 110 having an outputshaft 111 connected to gears 109, one of which gears is coupled to teeth108 formed in the wall of the probe 107 or a rack connected thereto.Thus, depending on the direction of rotation of the shaft 111 of motor110, and the time of operation of said motor, the location of the probe104 within the mold cavity 103 may be predeterminately controlled.

Four types of transducing means are illustrated in FIG. 8, two of whichare mounted in the probe 104 and have been described. The transducer 125is connected by means of suitable lines 126 to an ultrasonic energygenerator 127 such as a high-frequency oscillator of suitable knowndesign operative to vibrate the transducer in the range of 20 to 100kilocycles or higher for imparting suitable desired vibrations to themolding material through the probe. Notation 127F and 127S refer to onand off controls for the oscillator or generator 127 which controls arerespectively connected to lines extending from the master controller 134to operate and shut down the generator 127. Wherever utilized, thenotation PS refers to a suitable source of electrical energy. It isassumed that one or more sources of electrical energy are connected toall of the components illustrated in FIG. 8 requiring same, whetherillustrated or not, to provide suitable operation of said components.

Shown operatively coupled to the side wall 100 of the mold 99 is a firsttransducer 130 which may be made in accordance with any of the describedstructures and may comprise one or more piezo electric ultrasonictransducers for imparting ultrasonic energy through the wall of the moldto the molding material or one or more coils of electrical conductingwire for generating intense magnetic fields or induction energy which isapplicable, as described, to the molding material in the mold cavity103.

In other words, the notation 130 is symbolic and refers to what maycomprise one or more of the same type of transducer or a plurality ofdifferent types of transducers properly disposed within and/or about thewall of the mold. The transducer 130 is operatively connected to agenerator 132 of suitable electrical energy through lines 131. Thesource 132 contains on-off controls denoted 132F and 132S connecting itwith a power supply PS for energizing same. The device 132 may comprisea suitable oscillator if the transducer 130 is an ultrasonic transduceror a power supply or transformer for providing suitable electricalenergy to energize the transducer 130 for generating magnetic orinduction energy, as described.

Also shown in FIG. 8 is a second transducer 135 which is operativelycoupled to the bottom wall of the mold for imparting similar ordifferent energy than that generated by transducer 130 to the moldingmaterial disposed in the mold cavity. The transducer 135 may thuscomprise one or more piezo electric transducers, magnetic coils, orinduction means associated with the bottom or side walls of the mold ashereinbefore described and may be operated concurrently or in sequencewith the operation of the transducer 130 to apply the same or differenttypes of wave energy to the solidifying molding material disposed in themold cavity.

Turning now to the master controller 134, which may comprise, asdescribed, an analog or digital computer or, in a simpler form, a presetor preprogrammed, self-recycling multi-circuit timer. Such amulti-circuit timer may be made in accordance with the teachings of suchpatents as U.S. Pat. No. 2,580,787, U.S. Pat. No. 1,172,080 and othersknown in the art operative for carrying out a predetermined program ofoperations by closing and opening one or more electrical circuits atpredetermined times during a cycle of operations. In its simplest form,the device 34 may comprise a shaft driven by a constant speed electricalmotor and containing space-separated cams which are so located on saidshaft as to open and close various contacts or switches duringpredetermined times in the rotation of the shaft for predeterminatelycontrolling the motors, solenoids and switches associated with thecomponents of the system described for attaining the desired describedresults.

While separate high frequency electrical generators may be utilized asshown for driving each of the probe and mold wall mounted transducersdescribed a single oscillator may be utilized to drive two or more, ifnot all of the transducers simultaneously, or in sequence. A variablefrequency oscillator may also be provided for driving one or more of thedescribed transducers in a in a preprogrammed or adaptive control modeof operation.

For most polymers and metals, apparatus of the type described hereinwhich utilizes ultrasonic wave energy to control crystal growth andimprove or refine grain structure of the metal may be operated in thefrequency range of 20 to 100 kilocycles per second or greater and in thepower range of 50 to 500 watts depending on the effects desired and thecross section of the molding, casting or extrusion subjected to suchultrasonic radiation. Crystal orientation and grain refining will beimproved with increasing power input to the solidifying melt. Theapplication of vibratory energy, whether ultrasonic or subsonic, as wellas the application of other forces such as intense magnetic fields,should be applied to the melt just above the solidification temperature,say 150° to 300° F. above the solidification temperature of metal andcontinued to solidification. In refining aluminum and its alloys, forexample, the vibrational energy or oscillating magnetic field may beapplied to the molten material of the molding or that portion of thecontinuous casting which is at a temperature in the range of 1250° F. to1300° F. and continued to or beyond solidification at approximately1000° F.

Ultrasonic and subsonic waves may be simultaneously or sequentiallyapplied to the solidifying material per se, or simultaneously orsequentially with the application of an intense oscillating (expandingand collapsing) magnetic field to the molding or casting as described toimprove grain and crystal structure of plastics, metals and certainceramic materials. The intensity of the magnetic field generated in themold and casting or other shape will depend on the size of the molding,forging or casting being treated by the intense magnetic field generatedby the magnetic coil situated in or about the mold. In general, magneticfields in the range of 100 to 1000 kilogauss will suffice to grainrefine most ferrous and non-ferrous metal shapes and serve tosubstantially reduce or eliminate the porosity thereof as well as toorient and control crystal growth. Lower intensity constant and/orintermittently generated magnetic fields (10 to 100 kilogauss) may beemployed to control crystal growth in polymeric and ceramic materials.

In FIG. 8 notations 131 and 136 refer to cables extending from suitablesources of alternating electrical energy 132 and 137 to transducers 130and 135 coupled to the side and bottom walls of mold 99. On and offcontrols denoted 132F, 132S, 137F and 137S for the oscillators 132 and137 and are connected to respective outputs of the master controller ormulti-circuit timer 134 and may comprise respective inputs of respectivebi-stable switches pulsed by signals received from said mastercontroller.

Also shown in FIG. 8 is an apparatus 138 for controllably addingmaterial to the molding material preferably as the latter is deliveredto the mold through the pour spout or injection nozzle 117. Theapparatus 138 includes one or more pour spouts or injection nozzles 139and means 140 for controllably delivering said material or a pluralityof materials either into the stream of molding material flowed throughspout 117 or the mold itself. The additive may comprise a liquid ormolten plastic or metal, hard particles, short filaments, whiskers, etc.or combinations of such materials which are premixed or delivered fromseparate nozzles or injectors. Accordingly, dependent on what form theadditive material is in, delivery means 140 may comprise a controlledpump, solenoid valve, vibrator, belt conveyor or control means forpressurized gas operative to carry the additive. Notation 141 refers toa controlled motor for operating the pump or conveyor 140 in response tosignals received on its inputs 141F and 141S from the master controller134. Motor 141 may also be variably controlled in its operation bysuitable analog and/or digital control signals generated by the mastercontroller 134 and applied to a digital or analog controller as definedin U.S. Pat. Nos. 3,412,431 and 3,422,648. In other words, means areprovided in the apparatus of FIG. 8 for variable controlling the rate offlow of additive material to the molding material in the mold and thetiming of the admission of said material if such variables are requiredto produce moldings or castings having predetermined physicalcharacteristics. Since the timing of the flow of additive is alsocontrollable, articles may be produced by means of the apparatus of FIG.8 which vary in physical characteristic or additive content throughoutthe article.

It is noted that the motor 120 controlling operation of pump 118 mayalso be variably controllable in its operation and controlled in apreprogrammed manner by suitable digital or analog command controlsignals generated by the master controller and applied as disclosed inmy U.S. Pat. Nos. 3,412,431 and 3,422,648. If one or a plurality ofadditives are also admitted or injected into the mold in a varablycontrolled manner, as described, by means of command control signalsgenerated by the master controller 134 and the other variables such asultrasonic energy generation and transmission, rate of flow of coolantthrough the mold wall, etc. are also variably controllable by signalsgenerated on respective outputs of the master controller 134, then theapparatus of FIG. 8 may be automatically operated to accommodate avariety of different molds, molding materials and additives to formarticles or castings having wide ranges of physical characteristics.

The apparatus of FIG. 8 may be employed to provide new and improvedsingle and continuous castings of metal which are dispersionstrengthened with fine particles of ceramic material which are disposedpeppered throughout the microstructure of the casting in a uniform orvariably predetermined density as determined by properly programming themaster controller 134 to control metal and particle flow, mold and metalvibration and cooling rate. Nickel and nickel-chromium alloys of variouscomposition may be cast or injection molded as described with fineparticles of thorium oxide 0.0001 to 0.00001 inches in diameter added tothe poured or injected metal or the melt in the mold by the means ofFIG. 8 to substantially improve the strength of the metal composite soproduced at high temperatures. The employment of vibrations and/ormagnetic field energy as described may be effected during the additionof the ceramic particles to uniformly or otherwise predeterminatelydisperse the particles in the casting. The application of said energy orenergies may also be used to improve the macro and micro-structures ofthe metal casting or molding while simultaneously uniformlypredeterminately dispersing said particle in the casting. For example,the application of said energy may be used to align the metal crystalsor grains and grain boundaries falling along the major stress axis ofthe casting or molding providing a columnar grain structure which willimprove the high temperature properties of the casting.

Carbon or graphite filaments, ceramic fibers such as boron nitride,aluminum oxide, metal crystals such as whiskers and the like may also beadded to and dispersed within or predeterminately located in the castingby automatically controlling the flow and or position of the dispensingnozzle or nozzles 139 by means of signals generated by the mastercontroller 134 as described.

The apparatus of FIG. 8 may be operated to effect controlledsolidification patterns in castings and moldings by differentially andpredeterminately heating the mold or die 99 with or without theapplication of auxiliary energy as described. For example, a pluralityof pumps similar to pump 121 and respective driving motors controlled intheir operation by signals generated by the master controller 134 asdescribed, may each be operative to control the flow of coolant liquidto different passageways in different portions of the wall of the moldor die 99. By thus differentially cooling the wall of the mold so thatmetal solidification is made to advance as a uniform front along theaxis of the casting, the grain boundaries are made to line up along themajor stress axis. By properly controlling the flow of heat transferfluid, as described, during the casting procedure monocrystallinecastings may be produced having superior physical characteristics attemperature. The use of vibrational energy as described may be employedto assist in the formation of such monocrystalline structures.

It is noted that the apparatus hereinbefore described may also beoperated to improve the physical properties of castings in the die ormold in which they are cast by so called strain hardening effected bypredeterminately applying vibrational forces to the mold by means of thetransducers described and/or by the application of strain energy to thecasting during and after its solidification while still in the mold bythe described magnetic coil means surrounding the mold which areenergized and deenergized one or more times to apply forces to the moldand casting which subject the casting to the strain hardeningdeformation.

The apparatus hereinabove described and particularly that illustrated inFIG. 8 may also be utilized to provide a coarsegrained microstructure inmetal alloys containing dispersion strengthening components therebyproviding strength for the alloy at a wider range of temperatures thanwould ordinarily be experienced during the alloying steps effected byconventional means. For example, when aluminum and titanium are added toNi-Cr-ThO₂ intermediate temperature strength (1200 F.) is increased butthe strength of the alloy at 2000 F. is little improved due to theprecipitation of the Ni₃ (Al,Ti) phase which prevents the microstructurefrom becoming coarse grained. While thermomechanical treatment resultingfrom controlled heating and cooling of the alloy has little effect onimproving the grain structure, the application of ultrasonic vibrations,as described, during and immediately after alloying and particularlywhile the alloy is cooling may be utilized to provide a coarse grainedmicrostructure so as to provide an increase in strength of thedispersion hardened alloy at low, intermediate and high temperatures.The apparatus described and illustrated in FIG. 8 may also be utilizedto predeterminately produce alloys and dispersion hardened metals byprogram controlling the flow of two or more alloying metals andparticles such as thorium oxide, titanium carbide, aluminum oxide andother materials to an alloying chamber or crucible, controllingtemperature of the melt and controlling ultrasonic vibrations during theaddition and hardening phases of alloying and predeterminately varyingthese variables during a cycle to provide a metal alloy which ispredeterminately composed, predeterminately dispersed with particles andof predetermined grain or crystalline microstructure.

The apparatus described may also be utilized to produce new alloyshaving predetermined microstructures. For example, fine grains of carbon0.0001 to 0.00001 inches in diameter) may be dispersed uniformlythroughout iron, steel, nickle, copper, aluminum and other metals aswell as alloys of these metals and/or may be disposed along the grainboundaries of course grained microstructure to improve the physicalcharacteristics thereof. Said carbon may comprise pyrolitic graphite orother forms of graphite which will maintain its granular identity at thetemperature required for alloying or melting and dispersing same in themelt. Similar fine grains of other ceramic materials such as rutheniumdioxide may be similarly dispersed in the melt of such metals or variousalloys thereof, per se or in combination with other particles by theapplication of ultrasonic energy to the melt and solidifying metal bythe means described. Since ruthenium dioxide is unusually stable and iselectrically conductive and oxidation resistant, it may be used to bothdispersion harden and improve the electrical conductivity of variousmetals and alloys such as ferrous metals and alloys, aluminum alloys,certain copper alloys such as titanium copper and zirconium copper,beryllium copper and other beryllium alloys, tungsten and titanium metaland alloys, etc. Controllably energized coils disposed in the wall ofthe mold and/or the probe may also be utilized to generate intensemagnetic fields in the molding material to predeterminately align orotherwise dispose particles or filaments as described in the finalcasting or molding. Ruthenium dioxide, for example, which iselectrically conductive, may be positionally controlled and alignedwithin the casting or molding by magnetic field forces applied bymagnetic coils surrounding the mold, disposed in the mold wall ordisposed in the probe.

The apparatus described or modifications thereof may also be utilizedfor molding particulate materials to shape such as metal or plasticpowders which are compacted in the mold by means of the probe and workedby a combination of probe movement and vibrations imparted through theprobe and mold walls as described. Magnetic and induction energy mayalso be applied to compress and heat the particles in the mold in apredetermined manner as defined by the signals generated by mastercontroller 134, so as to either render said particles in a molten orsintered condition. The ultrasonic and magnetic vibrations described maybe utilized to predeterminately compact and control the macro and microstructure of the material worked by the probe or male mold member in themold.

In another form of the invention, the material admitted to the mold maycomprise a monomer such as a synthetic plastic monomer per se, may bemixed with a monomer or contain a monomer coated thereon. For example,particles or filaments may be admitted to the mold which are eitherprecoated with a plastic monomer or coated in the mold with a monomeradmitted thereto as a liquid or vapor. Ultrasonic energy imparted to themonomer through the probe 104 and/or the mold walls may be operative topolymerize the monomer thereby either forming a solid shape thereof orbonding the particles or filaments together into a solid or porous mass.

Ultrasonic energy generated in the probe or transducers mounted in themold wall or surrounding the mold may also be utilized to either effector assist in the production of carbonized material in the mold or die.For example, carbonizable material such as a suitable plastic polymercontaining a hydrocarbon such as acrylonitrile resin, may be carbonizedper se in the mold by heating the mold and transmitting ultrasonicenergy thereto as described or may be formed as an extrusion orextrusions passing through the mold by heat applied to the mold wall andultrasonic energy applied thereto through the probe or mandrel and/ormold walls. Particles coated with a monomer or polymer may bepolymerized and carbonized in the mold by means of heat and ultrasonicenergy applied to the mold and probe as described.

To effect the forms of the invention described above, the ultrasonicenergy may be applied in the range of 20 to 200 k.c.s. and the heat atthe temperature required to carbonize the particular polymer. Intensemagnetic field energy may be generated in coils surrounding the moldwall or within the probe and operative to expand and contract the moldwalls, probe and/or solid material disposed within the mold such asparticles, filaments, chips and the like or solidified molten moldingmaterial so as to work the latter and improve it macro and/ormicro-structure.

If the mold described is a die employed to effect the continuous castingor extrusion of the material fed thereto to shape, the probe maycomprise a mandrel for shaping the interior of the casting or extrusionand the generation of one or more forms of vibrational energy therein bythe means described may serve not only to improve and predetermine theinternal structure of the casting or extrusion but also to reduce theforce required to pull the casting from the mold or force extrusionmaterial through the die. Similarly, vibrational energy applied to thewalls of the mold or die may also be operative to improve internalstructure of the molding, casting or extrusion and to reduce the forcerequired to extrude or remove the casting from the die. The formation ofcomposite extrusions or castings involving the coating of one materialon a core material may also be facilitated by ultrasonic and/or magneticfield energy applied as described and operative to perform one or moreof the functions of facilitating extrusion or casting as described,improving the physical characteristics of the core material, improvingthe physical characteristics of the coating material, improving the bondbetween the core and coating material by welding, molecularly bonding orcausing the material of either to penetrate the surface stratum of theother. If the coating is a monomer, it may be polymerized as it isdisposed against the core material by ultrasonic energy applied asdescribed herein.

What is claimed is:
 1. A molding method comprising:(a) controllablyflowing a fluent molding material to a cavity of a mold, (b) receivingand shaping a select quantity of said fluent molding material in adefined configuration in said mold cavity, (c) sensing temperature ofthe molding material and generating a feedback signal indicativethereof, (d) transferring heat with respect to said mold and saidmolding material in said mold to cause said select quantity of saidmolding material to solidify in said mold, (e) analyzing said feedbacksignal indicative of the temperature associated with the moldingmaterial with a computer and controlling the heat transferred withrespect to said mold in a select manner in response to the analyzedfeedback signal.
 2. A method in accordance with claim 1 wherein saidcomputer controls acts (a) and (e) and the flow of said molding materialis controlled in response to said feedback signal.
 3. A method inaccordance with claim 2 further including controlling the rate of heattransferred with respect to said mold in response to said feedbacksignal.
 4. A method in accordance with claim 1 wherein the computer isemployed to receive and analyze said feedback signal to effect controlof the acts in parts (a) and (e).
 5. A method in accordance with claim 1wherein the acts in part (d) are effected by controlling the rate ofheat transferred with respect to said mold.
 6. A method in accordancewith claim 1 wherein the acts in part (d) are effected by controllingflow of a heat transfer fluid through said mold.
 7. A method inaccordance with claim 1 wherein the acts in part (d) are effected bycontrolling the flow of said molding material into said mold.
 8. Amethod in accordance with claim 1 wherein the acts in part (d) areeffected by controlling the flow of said molding material into said moldand flow of heat transfer fluid with respect to said mold.
 9. A methodin accordance with claim 1 including responding to said feedback signalby controlling the rate of heat transferred with respect to said mold.10. A method in accordance with claim 1 including responding to saidfeedback signal by controlling the rate of flow of said molding materialinto said mold.
 11. A method for molding comprising:a) flowing a fluentmolding material to a cavity of a mold; b) receiving and shaping aselect quantity of said fluent material into a defined configuration insaid mold cavity; c) generating first control signals which are appliedby operating a master controller to control the transfer of heat withrespect to said molding material for predeterminately controlling thetemperature of the molding material as it flows into and is retainedwithin said mold; d) simultaneously as said first control signals aregenerated and applied to control the temperature of said moldingmaterial, generating second control signals; and e) applying said secondcontrol signals to control the flow of said molding material to saidmold cavity.
 12. A method in accordance with claim 11 wherein said firstand second control signals are generated on an output of a mastercontroller.
 13. A method in accordance with claim 12 wherein said mastercontroller is a computer generating said first and second controlsignals on an output means thereof.
 14. A method in accordance withclaim 11 wherein said first and second control signals are concurrentlygenerated with respect to each other.
 15. A method of molding inaccordance with claim 11 wherein the second control signals aregenerated by sensing a temperature that is related to temperature ofsaid molding material flowed to said cavity.
 16. A method for moldingcomprising:(a) flowing a fluent molding material to a cavity of a mold;(b) receiving and shaping a select quantity of said fluent material intoa defined configuration in said mold cavity; (c) generating firstcontrol signals which are applied by operating a master controller tocontrol the transfer of heat with respect to said molding material forpredeterminately controlling the temperature of the molding material asit flows into and is retained within said mold by sensing temperature ofsaid molding material flowed to said cavity and generating feedbacksignals relating to the sensed temperature and:i) electrically comparingsaid feedback signals with reference signals indicative of desiredmolding material temperature; ii) generating difference signals inresponse to the compared feedback and reference signals; and iii)applying said difference signals to variably effect the flow of a heattransfer material to controllably transfer heat with respect to a wallof said mold; d) simultaneously as said first control signals aregenerated and applied to control the temperature of said moldingmaterial, generating second control signals; and e) applying said secondcontrol signals to control the flow of said molding material to saidmold cavity.
 17. A method for molding comprising:a) flowing a fluentmolding material to a cavity of a mold; b) receiving and shaping aselect quantity of said fluent material into a defined configuration insaid mold cavity; c) generating first control signals which are appliedby operating a master controller to control the transfer of heat withrespect to said molding material for predeterminately controlling thetemperature of the molding material as it flows into and is retainedwithin said mold; d) simultaneously as said first control signals aregenerated and applied to control the temperature of said moldingmaterial, generating second control signals by:i) generating referencesignals indicative of desired cyclical flow of molding material during amolding cycle; ii) sensing flow of molding material to said mold cavityduring a molding cycle and generating feedback signals; iii)electrically comparing said feedback signals and said reference signals;iv) generating difference signals in response to the compared feedbackand reference signals; and v) applying said difference signals togenerate said second control signals which control the flow of saidmolding material to said mold cavity; and e) applying said secondcontrol signals to control the flow of said molding material to saidmold cavity.
 18. A molding method comprising:(a) controllably flowing afluent molding material to a cavity of a mold; (b) receiving and shapinga select quantity of said fluent molding material into a definedconfiguration in said mold cavity; (c) sensing temperature of themolding material and generating a feedback signal indicative thereof;(d) transferring heat with respect to said mold and the molding materialin the mold to cause said select quantity of said molding material tosolidify in said mold; (e) receiving said feedback signal indicative oftemperature associated with the molding material; and (f) operating acomputer to produce signals for controlling the heat transferred withrespect to said mold in response to said feedback signal.
 19. A moldingmethod in accordance with claim 18 wherein said computer also controlsan additional molding variable.
 20. A molding method in accordance withclaim 19 wherein said additional molding variable is a rate of flow ofmaterial to the cavity mold.
 21. A molding method comprising:(a)controllably flowing a fluent molding material to a cavity of a mold;(b) receiving and shaping a select quantity of said fluent moldingmaterial into a defined configuration in said mold cavity; (c) sensingtemperature associated with the molding material and generating afeedback signal indicative thereof; (d) transferring heat with respectto said mold and the molding material in said mold to cause said selectquantity of said molding material to solidify in said mold; (e)receiving said feedback signal indicative of the temperature associatedwith the molding material and operating a computer to produce signalsfor controlling the heat transferred with respect to said mold in aselect manner in response to said feedback signal; and (f) sensing flowof said molding material and generating feedback signals of the sensedflow to control said flow.
 22. A molding method in accordance with claim21 wherein both feedback signals are compared with reference signalsgenerated by said computer.
 23. A molding method comprising:(a)controllably flowing a fluent molding material to a cavity of a mold;(b) receiving and shaping a select quantity of said fluent moldingmaterial into a defined configuration in said mold cavity; (c) sensingtemperature associated with the molding material being fed to the moldand generating a feedback signal indicative thereof; (d) transferringheat with respect to said mold and the molding material in said mold tocause said select quantity of said molding material to solidify in saidmold; (e) receiving said feedback signal indicative of the temperatureassociated with the molding material and operating a computer to producesignals for controlling the heat transferred with respect to saidmolding material in a select manner in response to said feedback signal;and (f) sensing flow of said molding material and generating feedbacksignals of the sensed flow to control said flow.
 24. A molding method inaccordance with claim 23 wherein both feedback signals are compared withreference signals generated by said computer.
 25. A molding methodcomprising:(a) controllably flowing a fluent molding material to acavity of a mold; (b) receiving and shaping a select quantity of saidfluent molding material into a defined configuration in said moldcavity; (c) sensing temperature of the molding material and generating afeedback signal indicative thereof; (d) transferring heat with respectto said mold and the molding material in the mold to cause said selectquantity of said molding material to solidify in said mold; (e)receiving said feedback signal indicative of temperature associated withthe molding material; and (f) operating a computer to produce signalsfor controlling the flow of the molding material to said mold cavity inresponse to said feedback signal.
 26. A molding method in accordancewith claim 25 wherein the rate of molding material flow is controlled bysaid computer produced signals.